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Physics 1913

The Reflection of X-rays by Crystals

William Henry Bragg & William Lawrence Bragg

One whole-number rule, 2d sinθ = nλ, turns a crystal's X-ray reflections into the positions of its atoms.

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In depth · the introduction

Bounce X-rays off a crystal and, at just a few sharp angles, they flash back bright — and those angles tell you exactly how far apart the atoms are stacked.

The big idea

A crystal is atoms arranged in perfectly regular, repeating layers. Shine X-rays on it — light whose waves are about the size of an atom — and each layer acts like a faint mirror, reflecting a little of the beam. Most of the time the reflections from the many layers fall out of step and cancel, and almost nothing comes back. But at certain special angles every little reflection lines up in step and adds together into one bright beam.

Lawrence Bragg found the rule for those angles, and it is beautifully simple: twice the spacing between layers, times the sine of the angle, equals a whole number of wavelengths. Turn it around and the angle you measure hands you the spacing of the atoms. A measurement you can make from outside the crystal becomes a ruler for the inside.

How it came about

In 1912 Max von Laue showed that crystals scatter X-rays into a pattern of spots — proof in one stroke that X-rays are waves and that crystals are orderly atomic lattices. The pattern was striking but hard to read. A 22-year-old Cambridge student, William Lawrence Bragg, found a far simpler way to see it: picture the crystal as stacks of mirror-like layers.

His father, William Henry Bragg, a physics professor at Leeds, built the instrument to put the idea to work — an X-ray spectrometer that measured each reflection precisely. Father and son began reading crystal after crystal. In 1915 they shared the Nobel Prize in Physics; Lawrence, at 25, is still the youngest person ever to win it — though the shared honour partly hid how much of the key idea had been the son's.

Why it mattered

For the first time, people could find out where atoms actually sit. The Braggs showed that ordinary table salt contains no salt 'molecules' at all — just sodium and chlorine ions alternating in a grid — and mapped diamond, quartz and dozens of minerals. The technique they founded, X-ray crystallography, went on to reveal the structures of DNA, proteins, vitamins and medicines. Almost everything we know about the shapes of molecules began with bouncing X-rays off a crystal.

A way to picture it

Think of soldiers marching across a field ribbed with parallel ditches. If the ditches are spaced so that everyone steps over them in stride, the ranks stay together and march as one. Space them wrong and the ranks fall out of step and the column blurs. X-rays reflecting from atomic layers are like this: only when the extra distance down to the next layer is a whole number of wave-steps do all the reflections come back in unison — and shine.

Interactive X-ray diffraction: a beam strikes a stack of crystal planes spaced d apart at glancing angle θ and reflects; drag the angle, spacing and wavelength sliders and watch the reflected beam and a detector spot flash bright only at the special angles where the reflections line up in step.

Where it sits

This is the experimental partner to the era's atomic ideas. Dalton and Avogadro had argued that matter is made of atoms; the Braggs let us look at where those atoms are. Their X-ray pictures later supplied the dimensions of the DNA helix that Watson and Crick assembled, and grew into the whole field of structural biology — a line that runs from a salt crystal in 1913 all the way to today's prediction of protein shapes.

The original document
Original source text
W. H. Bragg & W. L. Bragg · Proceedings of the Royal Society of London A 88 (1913): 428–438
Background — von Laue's spots
In 1912 Max von Laue and his collaborators had passed X-rays through a crystal and recorded a regular pattern of spots, proving at once that X-rays are waves and that a crystal is a periodic lattice of atoms. The pattern, however, was awkward to interpret. This paper sets out a simpler and quantitative way to understand it.
The reflection picture
Lawrence Bragg's reframing is to treat the crystal as a stack of parallel planes of atoms, each plane acting as a weak mirror. The waves reflected from successive planes, separated by a spacing d, reinforce one another only when the extra distance travelled by the deeper wave is a whole number of wavelengths. With θ the glancing angle measured from the plane, that extra path is 2d sinθ, giving the reflection condition stated below.
2 d sin θ = n λ — the Bragg condition: n is the integer order, λ the X-ray wavelength, d the spacing between lattice planes, and θ the glancing angle measured from the plane.
The X-ray spectrometer
The elder Bragg's ionisation spectrometer makes the law usable: the crystal sits on a rotating table and an ionisation chamber on a movable arm measures the reflected intensity at each angle. As θ is swept, the reflection flares up at the Bragg angles; their positions fix the spacings d, and a set of reflections from different planes reconstructs the lattice. Run the other way, at a fixed crystal, the instrument sorts the beam's wavelengths — the crystal becomes an X-ray spectrometer.
Structures determined
The paper and its companions report the first crystal structures read this way — among them sodium chloride, potassium chloride, zinc blende and diamond — and draw the chemical conclusion that a rock-salt crystal contains no NaCl molecules: each ion is symmetrically surrounded by ions of the opposite kind in an extended ionic lattice.
[ … ]
The complete paper, with its measured reflection curves, indices and lattice dimensions, is available in full at the source below.
Royal Society of London · 1913